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Existing methods often focus on isolated user histories, neglecting the essential role of inter-user differences. We propose C-BPO, a framework that personalizes LLMs via preference-calibrated binary signals. By treating target user data as positive feedback and other users' data as an auxiliary set of implicit negative signals, C-BPO captures distinct inter-user differences. To mitigate the preference overlap issue, where shared task knowledge is erroneously penalized, we derive an objective grounded in Positive-Unlabeled (PU) learning theory. This approach purifies negative signals by subtracting ``positive bias'', ensuring alignment with unique idiosyncrasies without compromising general helpfulness. 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